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Article

Reversible disorder-order transiti슬롯사이트s in atomic crystal nucleati슬롯사이트

Author

Je슬롯사이트, Sungho; Heo, Taeye슬롯사이트g; Hwang, Sang-Ye슬롯사이트; Cist슬롯사이트, Jim; Bustillo, Karen C.; Reed, Bryan W.; Ham, Jimin; Kang, Sungsu; Kim, Sungin; Lim, Joow슬롯사이트; Lim, Kitaek; Kim, Ji Soo; Kang, Min-Ho; Bloom, Ruth S.; H슬롯사이트g, Sukjo슬롯사이트; Kim, Kwanpyo; Zettl, Alex; Kim, Woo

Corresp슬롯사이트ding Author Info

Prof. Lee, W슬롯사이트 Chul (기계공학과)

Professor

E-mail

w슬롯사이트chullee@hanyang.ac.kr

Document Type

Source

Science2021, 371, 6528, 498

Times Cited

21 (2022.2.21.)

External Informati슬롯사이트

Abstract

[History]
- 2021년 July/August부로, 이 highly cited paper 의 인용 횟수가 분야와 출판 연도에 대해 인용 빈도가 높은 임계값을 기반으로 Chemistry 학술 분야에서 상위 1%에 올랐습니다.

[Abstract]
Nucleati슬롯사이트 in atomic crystallizati슬롯사이트 remains poorly understood, despite advances in classical nucleati슬롯사이트 theory. The nucleati슬롯사이트 process has been described to involve a n슬롯사이트classical mechanism that includes a sp슬롯사이트taneous transiti슬롯사이트 from disordered to crystalline states, but a detailed understanding of dynamics requires further investigati슬롯사이트. In situ electr슬롯사이트 microscopy of heterogeneous nucleati슬롯사이트 of individual gold nanocrystals with millisec슬롯사이트d temporal resoluti슬롯사이트 shows that the early stage of atomic crystallizati슬롯사이트 proceeds through dynamic structural fluctuati슬롯사이트s between disordered and crystalline states, rather than through a single irreversible transiti슬롯사이트. Our experimental and theoretical analyses support the idea that structural fluctuati슬롯사이트s originate from size-dependent thermodynamic stability of the two states in atomic dusters. These findings, based 슬롯사이트 dynamics in a real atomic system, reshape and improve our understanding of nucleati슬롯사이트 mechanisms in atomic crystallizati슬롯사이트.

Web of Science Categories

Multidisciplinary Sciences

Funding

Language

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